Volume 50 Issue 5
May  2022
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WANG Xiao-xing, DUAN Yong-hong, ZHANG Jun-feng, TAN Yi-sheng. Catalytic conversion of CO2 into high value-added hydrocarbons over tandem catalyst[J]. Journal of Fuel Chemistry and Technology, 2022, 50(5): 538-563. doi: 10.1016/S1872-5813(21)60181-0
Citation: WANG Xiao-xing, DUAN Yong-hong, ZHANG Jun-feng, TAN Yi-sheng. Catalytic conversion of CO2 into high value-added hydrocarbons over tandem catalyst[J]. Journal of Fuel Chemistry and Technology, 2022, 50(5): 538-563. doi: 10.1016/S1872-5813(21)60181-0

Catalytic conversion of CO2 into high value-added hydrocarbons over tandem catalyst

doi: 10.1016/S1872-5813(21)60181-0
Funds:  The project was supported by the National Natural Science Foundation of China (21603258, 22172182) and the Natural Science Foundation of Shanxi Province (201601D202015)
  • Received Date: 2021-09-24
  • Accepted Date: 2021-11-05
  • Rev Recd Date: 2021-11-05
  • Available Online: 2021-12-17
  • Publish Date: 2022-05-24
  • The conversion of CO2, an abundant carbon resource, into high value-added chemicals or liquid fuels is an attractive way to mitigate carbon emissions, which is also a sustainable approach for the cyclic utilization of carbon resources. However, the selective activation and controllable conversion of CO2 is challenging because of the inertness of CO2 and high C–C coupling barrier. In recent years, some obvious breakthroughs on CO2 hydrogenation to high value-added chemicals or liquid fuels have been made by construction of a tandem catalytic system. For the tandem catalysis, the matching of Fe-based catalyst or metal oxides and zeolites, the assembly between the two active sites, the pore structure and acidity of the zeolites, as well as the reaction conditions and atmosphere all have important effects on the product distribution. Herein, the critical factors affecting the CO2 activation and conversion and the formation of the target products, as well as the stability over the tandem catalysts are summarized. Finally, an outlook is provided.
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