Review on the progress in the production of aromatic hydrocarbons by co-catalytic pyrolysis of biomass and plastics

HAN Dong; SUN Laizhi; CHEN Lei; YANG Shuangxia; LI Tianjin; XIE Xinping; XU Meirong; TANG Wendong; ZHAO Baofeng; SI Hongyu; HUA Dongliang

doi:10.1016/S1872-5813(23)60401-3

Volume 52 Issue 4

Apr. 2024

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Article Navigation > Journal of Fuel Chemistry and Technology > 2024 > 52(4): 481-495

HAN Dong, SUN Laizhi, CHEN Lei, YANG Shuangxia, LI Tianjin, XIE Xinping, XU Meirong, TANG Wendong, ZHAO Baofeng, SI Hongyu, HUA Dongliang. Review on the progress in the production of aromatic hydrocarbons by co-catalytic pyrolysis of biomass and plastics[J]. Journal of Fuel Chemistry and Technology, 2024, 52(4): 481-495. doi: 10.1016/S1872-5813(23)60401-3

Citation:

HAN Dong, SUN Laizhi, CHEN Lei, YANG Shuangxia, LI Tianjin, XIE Xinping, XU Meirong, TANG Wendong, ZHAO Baofeng, SI Hongyu, HUA Dongliang. Review on the progress in the production of aromatic hydrocarbons by co-catalytic pyrolysis of biomass and plastics[J]. Journal of Fuel Chemistry and Technology, 2024, 52(4): 481-495. doi: 10.1016/S1872-5813(23)60401-3

Citation:

HAN Dong, SUN Laizhi, CHEN Lei, YANG Shuangxia, LI Tianjin, XIE Xinping, XU Meirong, TANG Wendong, ZHAO Baofeng, SI Hongyu, HUA Dongliang. Review on the progress in the production of aromatic hydrocarbons by co-catalytic pyrolysis of biomass and plastics[J]. Journal of Fuel Chemistry and Technology, 2024, 52(4): 481-495. doi: 10.1016/S1872-5813(23)60401-3

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Review on the progress in the production of aromatic hydrocarbons by co-catalytic pyrolysis of biomass and plastics

doi: 10.1016/S1872-5813(23)60401-3

HAN Dong^1
,,
SUN Laizhi^{1
,
,},
CHEN Lei^1
,,
YANG Shuangxia^1
,,
LI Tianjin^1
,,
XIE Xinping^1
,,
XU Meirong^1
,,
TANG Wendong^2
,,
ZHAO Baofeng^1
,,
SI Hongyu^1
,,
HUA Dongliang^1
,

1.
Energy Research Institute of Qilu University of Technology (Shandong Academy of Sciences), Shandong Key Laboratory of Biomass Gasification Technology, Jinan 250014, China
2.
Shandong EMT New Material Co, Ltd, Dongying 257500, China

Funds: The project was supported by the Natural Science Foundation of Shandong Province (ZR2023MB040, ZR2022MB059, ZR2021QB156), the Key Research and Development Program of Shandong Province (2022CXGC010701), Shandong Province Science and Technology Small and Medium Enterprises Improvement Project(2023TSGC0460), Jinan City’s “20 New Colleges and Universities” project (202228018, 2021GXRC053), the Education and Industry Integration Innovation Pilot Project (2022JBZ02-03，2023PX086，2022PX009).

Received Date: 2023-08-03
Accepted Date: 2023-10-20
Rev Recd Date: 2023-10-20

Available Online: 2023-12-05

Publish Date: 2024-04-03

Abstract

Abstract

Aromatic hydrocarbons, especially monocyclic aromatic hydrocarbons such as benzene, toluene, and xylene (BTX), are important basic raw materials in the chemical industry, which are mainly derived from the catalytic reforming and thermal cracking of fossil fuels. The co-catalytic pyrolysis of biomass and plastic to produce aromatics has the advantages of high efficiency, environmental protection, low cost, and high selectivity. It can solve the problems of pyrolysis products such as high oxygen content, low aromatics yield, and low selectivity, which are caused by the characteristics of biomass rich in oxygen and poor in hydrogen. This article reviewed the research progress of co-catalytic pyrolysis of biomass and plastics to prepare aromatic compounds. Firstly, the types of raw materials for co-catalytic pyrolysis were introduced, and then the co-catalytic pyrolysis catalysts were emphasized. The reaction mechanisms of co-catalytic pyrolysis of biomass and plastics, such as the synthesis of dienes and hydrocarbon pool synergy were summarized. Finally, the future research focus and development direction of co-catalytic pyrolysis of biomass and plastics were proposed, which is developing the highly active and stable modified molecular sieve catalysts in order to improve the aromatics yield.
- biomass,
- plastic,
- co catalytic pyrolysis,
- aromatic hydrocarbon,
- catalyst

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References(74)

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